My favorite is Live & Let Die. He runs across alligator heads to escape! Does cinema get any better?
I like Craig, I think he's probably the most "true" to the books as far as the Bond character goes. I'm a fan of Roger Moore and Connery, although Connery's movies are so dated nowadays they're tough to watch sometimes.
I liked Timothy Dalton. I know he's much-maligned in Bond loving circles, but I thought Licence to Kill was a solid movie.